李留义

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发布时间:
2020-06-22
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李留义

姓名

李留义

学科

材料科学与工程

 

联系方式

电话:

***

Email:

lyli@fzu.edu.cn

个人主页:

https://orcid.org/0000-0002-3066-2991

地址:

福州大学国家大学科技园1号楼南909,邮编: 350108

个人简历

工作经历

2021.12-至今   福州大学 材料科学与工程学院  研究员,博导

2017.09-2021.12 福州大学 材料科学与工程学院  副研究员,

2009.04-2017.09 中国科学院福建物质结构研究所 副研究员

2007.03-2009.04 上海药明康德新药开发有限公司 合成研究员

教育经历

2013.09-2017.01 福州大学     光催化研究所  环境化学  博士

2004.09-2007.03 华中科技大学 化学化工学院  有机化学  硕士

教学情况

本科生《高分子材料基础》;硕士生《复合材料设计与制备》。

博士招生专业:材料物理与化学

硕士招生专业:材料科学与工程、材料化学、材料工程

研究领域

环境功能材料:新污染物降解

新能源材料:COFs材料光催化

主持项目

1. 国家自然科学基金面上项目,521721882022/1-2025/12结题

2. 福建省自然科学基金面上项目,2025J01471光催化全分解水功能导向的共价有机框架材料的设计制备及机理研究2025/092028/08在研

3. 福建省自然科学基金面上项目,2019J01226,基于主客体协同作用的COFs催化材料选择性光还原CO2研究,2019/4-2022/4,结题

4. 国家自然科学基金青年项目,21403238,基于Click反应的离子型多孔有机框架同步富集和催化转化CO2研究,2015/01-2017/12,结题

5. 福建省科技厅重点项目,2014H0053, 二氧化碳捕获与同步催化转化技术的研发,2014/11-2017/11,结题

 

论著成果

发表学术研究论文60多篇,授权中国发明专利20件。

发表论文

1. Zixian Guo, Youhang He, Mingfei Yu, Liuyi Li*, Jinhong Bi*, Yan Yu, Ling Wu*, Multiscale Engineering of COFs toward Practical Photocatalysis: From Heterojunction Design to Membrane Fabrication, Chinese Journal of Catalysis, 2026, DOI: 10.1016/S1872-2067(26)65055-3.

2. Qing Niu, Chentao Luo, Mingfei Yu, Liuyi Li*, Yan Yu*, Jinhong Bi*, Photoinduced Dynamic Electronic Asymmetry of Cu Dual-Atom Sites Within Covalent Organic Frameworks Boosts Hydrogen Production, Angew. Chem. Int. Ed., 2026, 65(14), e9127031.

https://doi.org/10.1002/anie.9127031

3. J. Huang, H. Yu, M. Yu, L. Li*, Y. Yu*, Ga alloying-induced electronic modulation of Pt synergized with COFs for boosting photocatalytic CO2 reduction, J. Mater. Chem. A, 2026, 14, 2849-2855.

https://doi.org/10.1039/D5TA07458D

4. Mingfei Yu, Junhan Huang, Qing Niu, Liuyi Li*, Yan Yu*, Jinhong Bi*, Asymmetric Structural Design in Cobaloxime-Integrated Covalent Organic Frameworks to Facilitate Photocatalytic Overall Water Splitting, Angew. Chem., 2025, 64 (22), e202504533 (VIP paper)

https://doi.org/10.1002/anie.202504533

5. Mingfei Yu, Wei Chen, Qingqing Lin, Liuyi Li*, Zheyuan Liu,  Jinhong Bi*, Yan Yu*, Electrostatic Confinement-Induced Excited Charge Transfer in Ionic Covalent Organic Framework Promoting CO2 Reduction, Angew. Chem., 2025, 64(6), e202418422

https://doi.org/10.1002/anie.202418422

6. Hongji Pan, Qing Niu, Mingfei Yu, Liuyi Li*, Yan Yu, Polarized π-Spacer Engineering Enables Sequential Electron Transfer for Photocatalytic Water Splitting in Covalent Organic Frameworks, ACS Energy Lett. 2025, 10(9), 4580-4588

https://pubs.acs.org/doi/10.1021/acsenergylett.5c02419

7. Jiangqi Ning, Qing Niu, Zheyuan Liu and Liuyi Li*, Aerobic Oxidation of Covalent Organic Framework Facilitating Photocatalytic CO2 Reduction with Water, Green Chem., 2025, 27, 6804  6812

https://pubs.rsc.org/en/content/articlelanding/2025/gc/d5gc01528f

8. Qing Niu, Wenfeng Deng, Yanlei Chen, Qingqing Lin, Liuyi Li*, Zheyuan Liu, Jinhong Bi*, Yan Yu*, Exciton Dipole Orientation and Dynamic Reactivity Synergistically Enable Overall Water Splitting in Covalent Organic Frameworks, ACS Energy Letters, 2024, 9, 5830-5835

https://pubs.acs.org/doi/full/10.1021/acsenergylett.4c02847

9. Rongbin Miao, Qing Niu, Liuyi Li*, Yan Yu, Ni-Metalized Covalent Organic Cage as a Photocatalyst for Selective Photoreduction of CO2 to CO, 2024, ChemSusChem, e202401699 (Hot Topic: Carbon Dioxide)

https://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/cssc.202401699

10. Jiangqi Ning, Junhan Huang, Yuhang Liu, Yanlei Chen, Qing Niu, Qingqing Lin, Yajun He, Zheyuan Liu, Yan Yu, Liuyi Li*, Alkyl-linked TiO2@COF heterostructure facilitating photocatalytic CO2 reduction by targeted electron transport, Chinese Journal of Structural Chemistry, 2024, 100453

https://www.sciencedirect.com/science/article/pii/S0254586124003350#appsec1

11. Mingfei Yu, Qiujun Li, Liuyi Li*, Yan Yu, Dual Cocatalysts on Covalent organic framework as Charge Transfer Mediator Facilitating Photocatalytic Water Oxidation, ChemCatChem, 2024, e202401154

12. Qing Niu, Wei Chen, Guodong Pan, Liuyi Li*, Yan Yu, Jinhong Bi, Ling Wu*, Jimmy C. Yu*, Spatially Separated Photoredox in a Covalent Organic Frameworks Heterostructure Boosting Overall Water Splitting, ACS Materials Lett., 2024, 6 (4), 14111417

13. Jiangqi Ning, Wei Chen, Qing Niu, Liuyi Li*, Yan Yu*,Charge Transport Approaches in Photocatalytic Supramolecular Systems Composing of Semiconductor and Molecular Metal Complex for CO2 Reduction, ChemSusChem, 2024, e202301963

https://chemistry-europe.onlinelibrary.wiley.com/doi/abs/10.1002/cssc.202301963

14. Haoming Huang, Qingqing Lin, Qing Niu, Jiangqi Ning, Liuyi Li*, Jinhong Bi, Yan Yu*, Metal- free photocatalytic reduction of CO2 on a covalent organic framework- based heterostructure, Chinese J. Catal., 2024, 60 201-208

15. Qiaoshan Chen, Yueling Chen, Mingfei Yu, Bin Xu, Houyi Wu, Liuyi Li, Jinhong Bi*, Modulating interfacial charges in CTF-based metal-insulator-semiconductor promotes selective CO2 reduction to CH4, Chemical Engineering Journal, 2024, 149027

16. Yajun He, Yun Zhao, Xiaofeng Wang, Zheyuan Liu*, and Yan Yu*, Liuyi Li*, Multiple Heteroatom-Hydrogen Bonds Bridging Electron Transport in Covalent Organic Framework-Based Supramolecular System for Photoreduction of CO2, Angew. Chem., 2023, 62(31), e202307160 (VIP paper)

https://onlinelibrary.wiley.com/doi/10.1002/anie.202307160

17. Yajun He, Guoyu Liu, Zheyuan Liu, Jinhong Bi*, Yan Yu*, Liuyi Li*, Photoinduced Hydration Boosts O2 Evolution on Co-Chelating Covalent Organic Framework, ACS Energy Letters, 2023, 8, 1857−1863

 https://pubs.acs.org/doi/10.1021/acsenergylett.3c00228

18. Huizhen Li, Yanlei Chen, Qing Niu, Xiaofeng Wang, Zheyuan Liu, Jinhong Bi, Yan Yu*, Liuyi Li*. The crystalline linear polyimide with oriented photogenerated electron delivery powering CO2 reduction. Chinese Journal of Catalysis, 2023, 49: 152-159.

https://www.cjcatal.com/CN/10.1016/S1872-2067(23)64450-X

19. Niu Qing, Mi Linhua, Chen Wei, Li Qiujun, Zhong Shenghong*, Yu Yan*, Li Liuyi*. Review of covalent organic frameworks for single-site photocatalysis and electrocatalysis. Chinese Journal of Catalysis, 2023, 50, 45-82. 

https://www.sciencedirect.com/science/article/pii/S1872206723644572

20. Guodong Pan, Xuesen Hou, Zheyuan Liu, Chengkai Yang, Jinlin Long, Guocheng Huang, Jinhong Bi, Yan Yu,* and Liuyi Li*, The Hydration-Initiated Pathway of Water Oxidation over Photoexcited Covalent Organic Frameworks, ACS Catal. 2022, 12, 14911−14917

https://pubs.acs.org/doi/10.1021/acscatal.2c03878

21. Yajun He, Guodong Pan, Liuyi Li,* Shenghong Zhong, Lingyun Li, Zheyuan Liu* and  Yan Yu,* Local Charge Transfer within a Covalent Organic Framework and Pt Nanoparticles Promoting Interfacial Catalysis. Catal. Sci. Technol. 2022, 12, 3240-3246

22. Guoyu Liu, Guodong Pan, Qiang Dang, Rui Li, Liuyi Li,* Chengkai Yang,* and Yan Yu*, Hollow Covalent Organic Framework Cages with Zn Ion-Implantation Promoting Photocatalytic H2 Evolution, ChemCatChem, 2022, e202101800

23. Qiang Dang, Hanlin Huang, Liuyi Li*, Xiaolin Lyu, Shenghong Zhong, Yan Yu*, and Dongsheng Xu*, Yolk-Shell-Structured Covalent Organic Frameworks with Encapsulated Metal-Organic Frameworks for Synergistic Catalysis, Chem. Mater. 2021, 33, 14, 5690–5699.

https://pubs.acs.org/doi/10.1021/acs.chemmater.1c01383

24. Wenjing Qiu, Yajun He, Liuyi Li,* Zheyuan Liu*, Shenghong Zhong, Yan Yu,* Donor-Acceptor Pairs in Covalent Organic Frameworks Promoting Electron Transfer for Metal-Free Photocatalytic Organic Synthesis. Langmuir, 2021, 37, 11535-11543.

https://pubs.acs.org/doi/10.1021/acs.langmuir.1c01801

25. Yajun He, Xin Chen, Chi Huang, Liuyi Li*, Chengkai Yang, Yan Yu*, Encapsulation of Co single sites in covalent triazine frameworks for photocatalytic production of syngas, Chinese J. Catal., 2021, 42, 123-130.

https://www.sciencedirect.com/science/article/pii/S1872206720636038

26. Shuhong Wu, Yi Pan, Huan, Lin, Liuyi Li, Xianzhi Fu, Jinlin Long*, Crystalline Covalent Organic Frameworks with Tailored Linkages for Photocatalytic H2 Evolution, ChemSusChem, 2021, 14 (22,) 4958-4972

27. Xin Chen, Qiang Dang, Rongjian Sa, Liuyi Li,* Lingyun Li, Jinhong Bi, Zizhong Zhang, Jinlin Long, Yan Yu,* Zhigang Zou*, Integrating Single Ni Sites into Biomimetic Networks of Covalent Organic Frameworks for Selective Photoreduction of CO2, Chemical Science, 202011(26), 6915-6922.

https://pubs.rsc.org/en/content/articlepdf/2020/sc/d0sc01747g

28. Xinyi Yang, Yajun He, Liuyi Li*, Jinni Shen, Jianhui Huang, Lingyun Li, Zanyong Zhuang, Jinhong Bi, Yan Yu*, One-Pot Fabrication of Pd Nanoparticles@Covalent Organic Framework-Derived Hollow Polyamine Spheres as a Synergistic Catalyst for Tandem Catalysis, Chem. Eur. J., 2020, ‏‏1864-1870.  (Hot paper) ‏‏

https://chemistry-europe.onlinelibrary.wiley.com/doi/pdf/10.1002/chem.201904731

29. Wanfu Zhong, Rongjian Sa, Liuyi Li*, Yajun He, Lingyun Li, Jinhong Bi, Zanyong Zhuang, Yan Yu*, and Zhigang Zou*, A Covalent Organic Framework Bearing Single Ni Sites as a Synergistic Photocatalyst for Selective Photoreduction of CO2 to CO, J. Am. Chem. Soc., 2019, 141(18), 7615-7621. (Highly cited paper)

https://pubs.acs.org/doi/pdf/10.1021/jacs.9b02997

30. Liuyi Li, Zhiming Zhou, Lingyun Li, Zanyong Zhuang, Jinhong Bi, Jinghe Chen, Yan Yu*, Jiaguo Yu*, Thioether-Functionalized 2D Covalent Organic Framework Featuring Specific Affinity to Au for Photocatalytic Hydrogen Production from Seawater, ACS Sustainable Chem. Eng., 2019, 7(22), 18574-18581.

https://pubs.acs.org/doi/pdf/10.1021/acssuschemeng.9b04749

31. Zhi ChengKaiyun ZhengGuiyun LinShengqiong Fang, Liuyi Li*, Jinhong Bi*, Jinni Shen and Ling Wu, Constructing a novel family of halogen-doped covalent triazine-based frameworks as efficient metal-free photocatalysts for hydrogen production, Nanoscale Adv., 2019, 1, 2674-2680.

32. Jinhong Bi,* Bin Xu, Long Sun, Huimin Huang, Shengqiong Fang, Liuyi Li,* Ling Wu, A Cobalt-Modified Covalent Triazine-Based Framework as an Efficient Cocatalyst for Visible-Light-Driven Photocatalytic CO2 Reduction, ChemPlusChem, 2019, 84(8),  1149-1154.

https://onlinelibrary.wiley.com/doi/10.1002/cplu.201900329

33. Kaixun Cui, Wanfu Zhong, Lingyun Li, Zanyong Zhuang, Liuyi Li*, Jinhong Bi, Yan Yu*, Well-Defined Metal Nanoparticles@Covalent Organic Framework Yolk-Shell Nanocages by ZIF-8 Template as Catalytic Nanoreactors, Small, 2019, 15(3), 1804419.

https://www.onlinelibrary.wiley.com/doi/full/10.1002/smll.201804419

34. Hong Zhong, Zixiao Hong, Can Yang, Liuyi Li, Yangsen Xu, Xinchen Wang and Ruihu Wang*, A Covalent Triazine-based Framework Consisting of Donor Acceptor Dyads for Visible-Light-Driven Photocatalytic CO2 Reduction, ChemSusChem, 2019, 12, 4493-4499.

35. Yujie Song, Hao Wang, Guangsheng Liu, Huan Wang, Liuyi Li, YanYu, Ling Wu*, Constructing surface synergistic effect in Cu-Cu2O hybrids and monolayer H1.4Ti1.65O4·H2O nanosheets for selective cinnamyl alcohol oxidation to cinnamaldehyde, J. Catal., 2019, 370, 461-469

36. Zhiming Zhou, Wanfu Zhong, Kaixun Cui, Zanyong Zhuang, Lingyun Li, Liuyi Li*, Jinhong Bi and Yan Yu*, A Covalent Organic Framework Bearing Thioether Pendant Arms for Selective Detection and Recovery of Au from Ultra-Low Concentration Aqueous Solution, Chem. Commun., 2018, 54, 9977-9980.

37. Zhi Cheng, Wei Fang, Tiansu Zhao, Shengqiong Fang*, Jinhong Bi*, Shijing Liang, Liuyi Li, Yan Yu, and Ling Wu, Efficient Visible-Light-Driven Photocatalytic Hydrogen Evolution on Phosphorus-Doped Covalent Triazine-Based Frameworks, ACS Appl. Mater. Interfaces, 2018, 10(48), 41415–41421.

38. Qianqian Jiang, Long Sun, Jinhong Bi*, Shijing Liang, Liuyi Li*, Yan Yu and Ling Wu, MoS2 Quantum Dots-Modified Covalent Triazine-Based Frameworks for Enhanced Photocatalytic Hydrogen Evolution, ChemSusChem, 2018, 22, 1108-1113.

39. Liuyi Li, Xiaofen Li, Zhi Cheng, Jinhong Bi*, Shijing Liang, Zizhong Zhang, Yan Yu and Ling Wu*, Rapid water disinfection over a Ag/AgBr/covalent triazine-based framework composite under visible light, Dalton Trans., 2018, 47, 7077-7082.

40. Yujie Song, HaoWang, ShijingLiang, YanYu, LiuyiLi, LingWu*, One-pot synthesis of secondary amine via photoalkylation of nitroarenes with benzyl alcohol over Pd/monolayer H1.07Ti1.73O4·H2O nanosheets, J. Catal., 2018, 361, 105-115.

41. Hao Wang, Yujie Song, Jinhua Xiong, Jinhong Bi, Liuyi Li, Yan Yu, Shijing Liang* and Ling Wu*, Highly selective oxidation of furfuryl alcohol over monolayer titanate nanosheet under visible light irradiation, Appl. Catal. B: Environ, 2018, 224, 394-403.

42. Siyi Guo, Yongrong Jiang, Liuyi Li, Xiangdong Huang, Zanyong Zhuang* and Yan Yu*, Thin CuOx-based nanosheets for efficient phenol removal benefitting from structural memory and ion exchange of layered double oxides, J. Mater. Chem. A, 20186, 4167-4178.

43.  href="#!" Zhubing Xiao, Liuyi Li, Yujiao Tang, Zhibin Cheng, Hui Pan, Dongxu Tian* and Ruihu Wang*, Covalent organic frameworks with lithiophilic and sulfiphilic dual linkages for cooperative affinity to polysulfides in lithium-sulfur batteries, Energy Storage Materials, 2018, 12, 252-259.

44. Zhitong Wang, Yujie Song, Junhua Zou, Liuyi Li, Yan Yu and Ling Wu*, The cooperation effect in the Au–Pd/LDH for promoting photocatalytic selective oxidation of benzyl alcohol, Catal. Sci. Technol., 2018, 8, 268-275.

45. Liuyi Li#, Lu Li#, Caiyan Cui, Hongjun Fan* and Ruihu Wang*, Heteroatom-doped carbon spheres from hierarchical hollow covalent organic frameworks precursors for metal-free catalysis, ChemSusChem, 2017, 22, 4921-4926.

46. Kaiqiang Jing, Jinhua Xiong, Na Qin, Yujie Song, Liuyi Li, Yan Yu, Shijing Liang* and Ling Wu*, Development and photocatalytic mechanism of monolayer Bi2MoO6 nanosheets for the selective oxidation of benzylic alcohols, Chem. Commun., 2017, 53, 8604-8607.

47. Liuyi Li, Wei Fang, Peng Zhang, Jinhong Bi*, Yunhui He, Jinyun Wang and Wenyue Su*, Sulfur-doped covalent triazine-based frameworks for enhanced photocatalytic hydrogen evolution from water under visible light, J. Mater. Chem. A, 2016, 4 (32), 12402-12406.

48. Liuyi Li, Caiyan Cui, Wenyue Su*, Yangxin Wang, and Ruihu Wang*, Hollow click-based porous organic polymers for heterogenization of [Ru(bpy)3]2+ through electrostatic interactions, Nano Res., 2016, 9(3): 779-786.

49. Liuyi Li, Huaixia Zhao, and Ruihu Wang*, Tailorable synthesis of porous organic polymers decorating ultrafine palladium nanoparticles for hydrogenation of olefins, ACS Catal., 2015, 5, 948-955.

50. Liuyi Li, Chunshan Zhou, Huaixia Zhao,and Ruihu Wang*, Spatial control of palladium nanoparticles in flexible click-based porous organic polymers for hydrogenation of olefin and nitrobenzene, Nano Res., 2015, 8, 709-721.

51. Liuyi Li, Huaixia Zhao, Jinyun Wang, and Ruihu Wang*, Facile fabrication of ultrafine palladium nanoparticles with size- and location-control in click-based porous organic polymers, ACS Nano, 2014, 8, 5352-5364.

52. Liuyi Li, Zhilin Chen, Hong Zhong, and Ruihu Wang*, Urea-based porous organic frameworks: effective supports for catalysis in neat water, Chem. Eur. J., 2014, 20, 3050-3060.

53. Liuyi Li, Jinyun Wang, Tao Wu, and Ruihu Wang*, Click ionic liquids: a family of promising tunable solvents and application in Suzuki-Miyaura cross-coupling, Chem. Eur. J., 2012, 18(25), 7842-7851.

54. Liuyi Li, Jinyun Wang, Chunshan Zhou, Ruihu Wang*, Maochun Hong, pH-Responsive chelating N-heterocyclic dicarbene palladium(II) complexes: recoverable precatalysts for Suzuki-Miyaura reaction in pure water, Green Chem., 2011, 13(8), 2071-2077.

55. Liuyi Li, Tao Wu, Jinyun Wang, Ruihu Wang*, Water-soluble ionic palladium complexes: effect of pendant ionic groups on palladium nanoparticles and Suzuki-Miyaura reaction in neat water, ChemPlusChem, 2014, 79, 257-265.

56. Liuyi Li, Lei Zhu, Dagui Chen, Xuelei Hu, and Ruihu Wang*, Use of acylhydrazine- and acylhydrazone-type ligands to promote Cu-catalyzed C-N cross-coupling reactions of aryl bromides with N-heterocycles, Eur. J. Org. Chem., 2011, 2692-2696.

57. Yangxin Wang, Hong Zhong, Liuyi Li and Ruihu Wang*, Facile synthesis and tunable porosities of imidazolium-based ionic polymers containing in situ formed palladium nanoparticles, ChemCatChem, 2016, 8(13), 2234-2240

58. Huaixia Zhao, Liuyi Li , Jinyun Wang and Ruihu Wang*, The spherical core-shell magnetic particles constructed by main-chain palladium N-heterocyclic carbenes, Nanoscale, 2015, 7 (8), 3532-3538

59. Huaixia Zhao, Xinxiong Li, Liuyi Li and Ruihu Wang*, Solvent-induced facile synthesis of cubic-, spherical- and honeycomb-shape palladium N-heterocyclic carbene particles and catalytic applications in cyanosilylation, Small, 2015, 11, 3642-3647

60. Jinhong Bi*, Wei Fang, Liuyi Li, Jinyun Wang, Shijing Liang, Yunhui He, Minghua Liu, Ling Wu*, Covalent triazine-based frameworks as visible light photocatalysts for the splitting of water, Macromol. Rapid. Comm. 2015, 36 (20), 1799-1805

61. Huaixia Zhao, Liuyi Li, Yangxin Wang, Ruihu Wang*, Shape-controllable formation of poly-imidazolium salts for stable palladium N-heterocyclic carbene polymers, Sci. Rep. 2014, 4, 5478.

62. Hong Zhong, Jinyun Wang, Liuyi Li and Ruihu Wang*, Copper-free Sonogashira cross-coupling reaction promoted by palladium complexes of nitrogen-containing chelating ligand in neat water at room temperature, Dalton, 2014, 43, 2098-2103.

63. Hong Zhong, Yaqiong Gong, Fengsen Zhang, Liuyi Li and Ruihu Wang*, Click-based porous organic framework containing chelating terdentate units and its application in hydrogenation of olefins, J. Mater. Chem. A, 2014, 2, 7502-7508.

64. Huaixia Zhao, Xinxiong Li, Jinyun Wang, Liuyi Li, Ruihu Wang*, Synthesis and crystal structures of coordination complexes containing Cu2I2 units and their application in luminescence and catalysis, ChemPlusChem, 2013, 78, 2098-2103.

65. Rui Lv, Yangxin Wang, Chunshan Zhou, Liuyi Li, Ruihu Wang*, Efficient copper-catalyzed ullmann reaction of aryl bromides with imidazoles in water promoted by a pH-responsive ligand, ChemCatChem, 2013, 5, 2978-2982.

66. Chunshan Zhou, Jinyun Wang, Liuyi Li, Ruihu Wang*, Maochun Hong, A palladium chelating complex of ionic water-soluble nitrogen-containing ligand: the efficient precatalyst for Suzuki-Miyaura reaction in water, Green Chem. 2011, 13, 2100-2106.